Thursday, September 22, 2016

HW 2: #3 Arsenic-life Bacterium

“‘Arsenic-life’ bacterium prefers phosphorus after all”, written by Daniel Cressey, discussed the debunking of a previous article posted in 2010. The article, “A Bacterium That Can Grow by Using Arsenic Instead of Phosphorus”, written by Felisa Wolfe-Simon & others, claimed that one of the bacteria in Mono Lake in California, which is very high in arsenic, could metabolize without phosphate and instead use arsenate. After several subsequent articles, this theory was proven to be false, and organisms need phosphate to grow. Specifically, an article published in October of 2012, “The molecular basis of phosphate discrimination in arsenate-rich environments” by Mikael Elias & others, tested to see how these bacteria even differentiate between the two extremely similar molecules. Being from the same group on the periodic table, phosphorous and arsenic have practically identical electronegativities and Van der Waals radii.
Image result for phosphorus atom vs arsenic atomImage result for phosphorus atom vs arsenic atom
This was the foundation for Wolfe-Simon’s article, but much of their results and findings were viewed subjectively because they wanted the outcome to be true. In the research done by Elias and his colleagues, they discovered that not only could these bacterial proteins differentiate between phosphate and arsenate, they did so through one key chemical bond. They all showed an extreme preference for phosphate, particularly the one bacterium that began this controversy which filtered in phosphate at levels of 4,500-fold the level of arsenate to phosphate. Arsenate was clearly still needed for these bacteria due to the lengths they went to in order to bond with all of the phosphates they could. However, some of the bacteria were able to bond with the arsenate after depleting the supply of phosphate, though the hydrogen bond was much weaker when the bacterium bonded with arsenate.
The (-)CAHB angles are optimal in the phosphate-bound structure but distorted with arsenate.
a. P. fluorescens PBP bound to phosphate has a more direct connection

b. P. fluorescens PBP bound to arsenate has an angled connection

Knowing that bonds could occur with arsenate when given no other option opens the door to the possibility that there may be life on other planets that survive without phosphate, or in fact use arsenate preferentially over phosphate. It would be interesting to test these, and other bacteria, in a pure arsenate solution, removing their ability to choose phosphate over arsenate.

Sources:
‘Arsenic-life’ bacterium prefers phosphorus after all: http://www.nature.com/news/arsenic-life-bacterium-prefers-phosphorus-after-all-1.11520
The molecular basis of phosphate discrimination in arsenate-rich environments: http://www.nature.com/nature/journal/v491/n7422/full/nature11517.html#supplementary-information
A Bacterium That Can Grow by Using Arsenic Instead of Phosphorus: http://science.sciencemag.org/content/332/6034/1163.full

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